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基础物理研究部

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姓名：董振超

联系邮箱：zcdong@ustc.edu.cn

教育经历

1987.5-1990.12  中国科学院福建物质结构研究所，物理化学专业，博士

1983.9-1987.4  厦门大学，物理化学专业，硕士

1979.9-1983.6  四川大学，物理化学专业，学士

工作经历

2021.12-至今  合肥国家实验室，高级研究员

2004.4 -至今  中国科学技术大学，教授

1996.1 -2004.3  日本国家材料科学研究所，主任研究官/主干研究员

1992.3 -1995.12  美国Iowa州立大学/Ames实验室，博士后研究助理

1990.12-1992.2  中国科学院福建物质结构研究所，助理研究员

研究简介

董振超长期从事单分子科学领域、特别是单分子光电效应的检测与调控方面的研究工作。他瞄准化学中物种识别的表征极限、光谱成像的极限分辨率、纳米环境中单分子的光电行为、以及分子间能量转移机制等前沿科学问题，通过研制高分辨扫描隧道显微镜与高灵敏光学技术相融合的联用系统，深入开展单分子尺度的光谱成像和局域场下的光电调控研究，取得了以下重要成果：

在国际上首次实现了亚纳米分辨的单分子拉曼光谱成像，颠覆了当时人们对光学成像分辨率极限和光场限域能力的认知；首次在单分子水平上实现了分子间偶极相干耦合作用的实空间观察，开辟了研究分子间相互作用和能量转移的新途径；首次展示了亚纳米分辨的单分子光致荧光成像，实现了近场荧光成像领域长期追求的在亚分子水平上用光“拍摄”场与物质相互作用的目标。相关成果发表于Nature、Science、Nature Photonics、Nature Nanotechnology、PRL、JACS等期刊。

核心研究方向‌：

1.‌单分子发光与相关光电子学研究

2.‌单分子拉曼散射与高分辨化学成像

3.‌单分子尺度能量转移与动力学研究

主要荣誉

2020  亚纳米分辨单分子光致发光成像成果入选“2020年度中国光学十大进展-基础研究类”

2018  中国真空学会“中国真空科技成就奖”

2016  国务院“政府特殊津贴”证书

2014  中国科学院“杰出科技成就奖（主要完成者）”

2013  亚纳米分辨拉曼成像成果入选“中国CAIA科技奖特等奖”、“中国科学十大进展”以及两院院士评选的“中国十大科技进展新闻”

2010  中国科学技术协会“全国优秀科技工作者”荣誉称号

代表性论文

[1] Zhu, R.#, Dong, X. R.#, Yang, B., Han, R. L., Mao, W., J., Chen, G.*, Zhang, Y., Zhang, Y.*, Dong, Z. C.*, Revealing single-molecule photocurrent generation mechanisms under on- and off-resonance excitation. Nano Letters, 25(1), 578-585 (2025).

[2] Han, Y.#, Dong, L.#, Zhu, L. Y.#, Hu, C. R., Li, H., Zhang, Y., Zhang, C.*, Zhang, Y.*, Dong, Z. C.*, Real-space spectral determination of short single-stranded DNA sequence structures. Journal of the American Chemical Society, 146(49), 33865-33873 (2024).

[3] Meng, Q. S.#, Zhang, J. X.#, Zhang, Y.*, Chu, W. Z., Mao, W. J., Zhang, Y., Yang, J. L., Luo, Y., Dong, Z. C.*, Hou, J. G.*, Local heating and Raman thermometry in a single molecule. Science Advances, 10(3), eadl1015 (2024).

[4] Luo, Y. #, Kong, F. F. #, Tian, X. J., Yu, Y. J., Jing, S. H., Zhang, C., Chen, G.*, Zhang, Y., Zhang, Y., Li, X. G., Zhang, Z. Y., Dong, Z. C.*, Anomalously bright single-molecule upconversion electroluminescence. Nature Communications, 15, 1677 (2024).

[5] Yang, B.#, Chen, G.#, Ghafoor, A., Zhang, Y. F., Zhang, X. B., Li, H., Dong, X. R., Wang, R. P., Zhang, Y., Zhang, Y., Dong, Z. C.*, Chemical enhancement and quenching in single-molecule tip-enhanced Raman spectroscopy. Angewandte Chemie International Edition, 62(13), e202218799 (2023).

[6] Itoh, T.*, Prochazka, M.*, Dong, Z. C.*, Ji, W., Yamamoto, Y. S., Zhang, Y., Ozaki, Y.*, Toward a new era of SERS and TERS at the nanometer scale: from fundamentals to innovative applications. Chemical Reviews, 123(4), 1552-1634 (2023).

[7] Kong, F. F.#, Tian, X. J. #, Zhang, Y.*, Zhang, Y., Chen, G., Yu, Y. J., Jing, S. H., Gao, H. Y., Luo, Y., Yang, J. L., Dong, Z. C.*, Hou, J. G.*, Wavelike electronic energy transfer in donor-acceptor molecular systems through quantum coherence. Nature Nanotechnology, 17(7), 729-736 (2022).

[8] Kong, F. F.#, Tian, X. J.#, Zhang, Y.*, Yu, Y. J., Jing, S. H., Zhang, Y., Tian, G. J.*, Luo, Y., Yang, J. L., Dong, Z. C.*, Hou, J. G., Probing intramolecular vibronic coupling through vibronic-state imaging. Nature Communications, 12, 1280 (2021).

[9] Xu, J. Y.#, Zhu, X.#, Tan, S. J.*, Zhang, Y., Li, B., Tian, Y. Z., Shan, H., Cui, X. F., Zhao, A. D., Dong, Z. C., Yang, J. L., Luo, Y., Wang, B.*, Hou, J. G.*, Determining structural and chemical heterogeneities of surface species at the single-bond limit. Science, 371(6531), 818-822 (2021).

[10] Wang, R. P.#, Yang, B.#, Fu, Q.#, Zhang, Y.*, Zhu, R., Dong, X. R., Zhang, Y., Wang, B., Yang, J. L., Luo, Y., Dong, Z. C.*, Hou, J. G.*, Raman detection of bond breaking and making of a chemisorbed up-standing single molecule at single-bond level. Journal of Physical Chemistry Letters, 12(7), 1961-1968 (2021)

[11] Yang, B.#, Chen, G.#, Ghafoor, A., Zhang, Y. F., Zhang, Y., Zhang, Y.*, Luo, Y., Yang, J. L., Sandoghdar, V., Aizpurua, J., Dong, Z. C.*, Hou, J. G.*, Sub-nanometre resolution in single-molecule photoluminescence imaging. Nature Photonics, 14(11), 693-699 (2020).

[12] Zhang, Y.#, Yang, B.#, Ghafoor, A., Zhang, Y., Zhang, Y. F., Wang, R. P., Yang, J. L., Luo, Y.*, Dong, Z. C.*, Hou, J. G.*, Visually constructing the chemical structure of a single molecule by scanning Raman picoscopy. National Science Review, 6(6), 1169-1175 (2019).

[13] Luo, Y.#, Chen, G.#, Zhang, Y.*, Zhang, L., Yu, Y. J., Kong, F. F, Tian, X. J, Zhang, Y., Shan, C. X., Luo, Y., Yang, J. L., Sandoghdar, V., Dong, Z. C.*, Hou, J. G.*, Electrically driven single-photon superradiance from molecular chains in a plasmonic nanocavity. Physical Review Letters, 122(23), 233901 (2019).

[14] Chen, G.#, Luo, Y.#, Gao, H. Y., Jiang, J., Yu, Y. J., Zhang, L., Zhang, Y., Li, X. G.*, Zhang, Z. Y.*, Dong, Z. C.*, Spin-triplet-mediated up-conversion and crossover behavior in single-molecule electroluminescence. Physical Review Letters, 122(17), 177401 (2019).

[15] Zhang, L.#, Yu, Y. J.#, Chen, L. G., Luo, Y., Yang, B., Kong, F. F., Chen, G., Zhang, Y.*, Zhang, Q., Luo, Y., Yang, J. L., Dong, Z. C.*, Hou, J. G.*, Electrically driven single-photon emission from an isolated single molecule. Nature Communications, 8, 580 (2017).

[16] Zhang, Y.#, Meng, Q. S.#, Zhang, L., Luo, Y., Yu, Y. J, Yang, B., Zhang, Y., Esteban, R., Aizpurua, J.*, Luo, Y., Yang, J. L., Dong, Z. C.*, Hou, J. G.*, Sub-nanometre control of the coherent interaction between a single molecule and a plasmonic nanocavity. Nature Communications, 8, 15225 (2017).

[17] Zhang, R.#, Zhang, X. B.#, Wang, H. F., Zhang, Y., Jiang, S., Hu, C. R., Zhang, Y., Luo, Y.*, Dong, Z. C.*, Distinguishing individual DNA bases in a network by non-resonant tip-enhanced Raman scattering. Angewandte Chemie International Edition, 56(20), 5561-5564 (2017).

[18] Richard-Lacroix, M.#, Zhang, Y.#, Dong, Z. C.*, Deckert, V.*, Mastering high resolution tip-enhanced Raman spectroscopy: towards a shift of perception. Chemical Society Reviews, 46(13), 3922-3944 (2017).

[19] Zhang, Y.#, Luo, Y.#, Zhang, Y.#, Yu, Y. J., Kuang, Y. M., Zhang, L., Meng, Q. S., Luo, Y., Yang, J. L., Dong, Z. C.*, Hou, J. G.*, Visualizing coherent intermolecular dipole-dipole coupling in real space. Nature, 531, 623-627 (2016).

[20] Liao, M. H., Jiang, S., Hu, C. R., Zhang, R., Kuang, Y. M., Zhu, J. Z., Zhang, Y., Dong, Z. C.*, Tip-enhanced Raman spectroscopic imaging of individual carbon nanotubes with subnanometer resolution. Nano Letters, 16(7), 4040-4046 (2016).

[21] Jiang, S., Zhang, Y., Zhang, R., Hu, C. R., Liao, M. H., Luo, Y., Yang, J. L., Dong, Z. C.*, Hou, J. G.*, Distinguishing adjacent molecules on a surface using plasmon-enhanced Raman scattering. Nature Nanotechnology, 10(10), 865-869 (2015).

[22] Duan, S., Tian, G. J., Ji, Y. F., Shao, J. S., Dong, Z. C., Luo, Y.*, Theoretical modeling of plasmon-enhanced Raman images of a single molecule with subnanometer resolution. Journal of the American Chemical Society, 137(30), 9515-9518 (2015).

[23] Zhang, R.# Zhang, Y.#, Dong, Z. C.*, Jiang, S., Zhang, C., Chen, L. G., Zhang, L., Liao, Y., Aizpurua, J., Luo, Y., Yang, J. L., Hou, J. G.*, Chemical mapping of a single molecule by plasmon-enhanced Raman scattering. Nature, 498(7452), 82-86 (2013).

[24] Zhu, S. E.#, Kuang, Y. M.#, Geng, F., Zhu, J. Z., Wang, C. Z., Yu, Y. J., Luo, Y., Xiao, Y., Liu, K. Q., Meng, Q. S., Zhang, L., Jiang, S., Zhang, Y., Wang, G. W.*, Dong, Z. C.*, Hou, J. G., Self-decoupled porphyrin with a tripodal anchor for molecular-scale electroluminescence. Journal of the American Chemical Society, 135(42), 15794-15800 (2013).

[25] Dong, Z. C.*, Zhang, X. L.#, Gao, H. Y.#, Luo, Y., Zhang, C., Chen, L. G., Zhang, R., Tao, X., Zhang, Y., Yang, J. L., Hou, J. G.*, Generation of molecular hot electroluminescence by resonant nanocavity plasmons. Nature Photonics, 4(1), 50-54 (2010).

[26] Dong, Z. C.*, Guo, X. L., Trifonov, A. S., Dorozhkin, P. S., Miki, K., Kimura, K., Yokoyama, S., Mashiko, S., Vibrationally resolved fluorescence from organic molecules near metal surfaces in a scanning tunneling microscope. Physical Review Letters, 92(8), 86801 (2004).

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